The increasing demand for aqueous energy storage (AES) solutions with high energy density, enlarged voltage windows, and extended cycling stability has spurred the development of advanced electrolytes. Redox-active molecules hold the promise for formulating aqueous electrolytes with enhanced electrochemical performance.
A dual redox-active (proton-conductive) electrolyte, containing Keggin-type phospohotungstate anions (PW12) and HQ, has been proposed for hybrid energy storage . The HQ molecules exhibited electrochemical activity in the positive electrode, while redox-active PW12 displays similar behavior in the negative electrode (Fig. 15A).
The ion migration through the ion conductor is necessary to enable the energy storage, but the metal pathways in the ion conductor need to be avoided. Based on the mechanism of resistive switching using ion conductors, their conductance can be precisely monitored as metal ions move in.
The inclusion of redox-active additives can stimulate mass-transfer behavior within the electric double layer . While the irreversible electrochemical process contributes to the formation of SEI layers on the electrode, the reversible redox reaction of molecules promotes energy storage within the aqueous system , .
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